RELATED: How to Copy Music to Your Android Phone You’ll need to manually copy your music library to Android instead. While iTunes will sync music files to iOS and iPadOS devices, it won’t do the same with Android devices. Unfortunately, Android doesn’t fit well into the Apple ecosystem. Manually Copy Your Music Files from iTunes to Android If you want your music available for offline playback, press the download icon in the “Songs” tab or in individual “Album” listings.